Peer-Reviewed Journal Details
Mandatory Fields
Biswas, S.; O’Regan, C.; Petkov, N.; Morris, M. A.; Holmes, J. D.
2013
September
Nanoletters
Manipulating the growth kinetics of vapor-liquid-solid propagated Ge nanowires
Published
Optional Fields
13
9
4044
4052

This article describes an innovative approach in which bimetallic alloy seeds of AuxAg1x are used to enhance the growth kinetics of Ge nanowires, via a vaporliquidsolid (VLS) growth technique. The decreased equilibrium concentration and increased supersaturation of Ge in the liquid alloy seeds, compared to pure Au seeds, results in favorable growth kinetics and the realization of high-aspect ratio millimeter-long Ge nanowires. Also detailed is the manifestation of the Gibbs-Thompson effect resulting in diameter-dependent nanowire growth rates as a function of the AuAgGe eutectic composition. Significantly, AuxAg1x alloy seeds lower the critical diameter of the Ge nanowires in this liquid-seeded growth approach. In situ TEM heating experiments established the correlation between the growth kinetics and equilibrium eutectic compositions in the ternary growth systems. The fundamental insights of nanowire growth demonstrated with the ternary eutectic alloys opens up opportunities to engineer the aspect ratio and morphology of a range of semiconductor nanowires.

Washington, DC, USA
na
na
http://pubs.acs.org/journal/nalefd
10.1021/nl401250x
Grant Details