Peer-Reviewed Journal Details
Mandatory Fields
Raha, S.; Srivastava, D.; Biswas, S.; Garcia-Gil, A.; Karttunen, A. J.; Holmes, J. D.; Singha, A.
2021
December
Applied Physics Letters
Probing lattice dynamics in ST12 phase germanium nanowires by Raman spectroscopy
Validated
WOS: 2 ()
Optional Fields
IN-SITU INTEGRATION DENSITY-OF-STATES HIGH-PRESSURE AMORPHOUS-SILICON CRYSTAL-STRUCTURE GE ANODES TRANSITIONS NANOCRYSTALS PARAMETERS
119
119
232105(1)
232105(7)
Germanium (Ge) plays a crucial role in setting up important functionalities for silicon-compatible photonics. Diamond cubic germanium is an extensively studied semiconductor, although its other exotic forms, like BC8, ST8, ST12 phases, may possess distinct electronic properties. We have fabricated stable ST12-Ge nanowires via a self-seeded bottom-up three phase growth in a confined supercritical toluene environment. Here, we report on the direct evidence of the presence of the ST12 phase by a combination of Raman spectroscopy and first-principles calculations using density functional theory (DFT). It is important to remark that the DFT calculation predicts all the Raman active optical phonon modes of the P 4 3 2 1 structure, and it is in very good agreement with the experimental results. The phonon dynamics as a function of temperature is investigated through Raman measurements at temperatures varying from 80 to 300 K. First-order temperature coefficients for all the observed Raman modes are estimated from the linear temperature dependence of the phonon shifts. A complete set of isobaric Gruneisen parameters is reported for all Raman modes of ST12-Ge nanowire, and the values are lower compared to the same for Si, dc-Ge bulk, and Ge nanowire. These results have important implications for understanding thermal properties of ST12-Ge nanowire.
MELVILLE
0003-6951
https://aip-scitation-org.ucc.idm.oclc.org/doi/10.1063/5.0066744
10.1063/5.0066744
Grant Details